面向国家洁净能源开发和“双碳”战略目标需求,开展太阳光催化全分解水制“绿氢”研究具有重要意义。近年来本课题组主要围绕“光催化全分解水制氢”中的关键科学问题开展系统研究:开发多个原创的窄带隙半导体材料体系,构筑高效异质结光催化剂,提出“界面层”调控助催化剂新策略,实现多个光催化全分解水制氢体系性能的大幅提升。主要包括开发的含氮半导体异质结体系刷新了当时表观量子效率(AQE)最高值以及创造了金属硫族化物基光催化Z机制全分解水AQE新纪录。现阶段,本课题组将主要围绕以下方面开展相关研究:
1. 窄带隙半导体材料的开发;
2. 光生电荷分离和转化的调控;
3. 光催化全分解水制氢体系的构筑。
陈闪山,博士,特聘研究员,博士生导师,国家级青年人才(海外)。近年来在太阳能-化学能转化领域取得了多项创新成果。发表SCI论文40余篇,其中第一作者或通讯作者在Nat. Rev. Mater., Joule (2篇), J. Am. Chem. Soc., Angew. Chem. Int. Ed. (2篇), ACS Catal.等期刊上发表SCI论文近20篇。授权国家发明专利3项。主持国家级青年人才和自然科学基金面上项目,参与了日本产业省人工光合成化学重大项目(ARPChem)、中日韩A3前瞻计划项目、国家863项目等。担任Frontiers in Nanotechnology期刊副主编、Chemistry - A European Journal和Chemical Synthesis客座编辑以及eScience, Chinese Chemical Letters青年编委,多次受邀担任业内专业期刊通讯评审人。
详见课题组网页:http://nankai.teacher.360eol.com/teacherBasic/preview?teacherId=5987&previewCode=
工作经历:
2021.2-至今, 南开大学, 材料科学与工程学院, 特聘研究员,博士生导师
2018.4-2020.11, 日本信州大学, 研究员, 合作导师:Domen Kazunari教授
2015.12-2018.3, 日本东京大学, 特任研究员, 合作导师:Domen Kazunari教授
学习经历:
2010.9-2015.5, 中国科学院大连化学物理研究所, 物理化学,博士,导师:李灿院士和章福祥研究员
2007.9-2010.6, 南京工业大学, 化学工程, 硕士, 导师:陆小华教授和杨祝红研究员
2003.9-2007.6, 合肥工业大学, 化学工程与工艺, 学士, 导师:崔鹏教授
申请-考核制博士生和博士后持续招生招聘中!!!
长期欢迎具有材料、光(电)催化、光谱背景的同学加入本课题组,共同成长与发展!有意者请直接联系陈闪山老师(sschen@nankai.edu.cn)。
[1] Shanshan Chen, Tsuyoshi Takata, Kazunari Domen*. Particulate photocatalysts for overall water splitting. Nat. Rev. Mater., 2017, 2, 17050. (Highly cited paper)
[2] Shanshan Chen, Chenyang Li, Kazunari Domen*, Fuxiang Zhang*. Particulate metal chalcogenides for photocatalytic Z-scheme overall water splitting. Joule, 2023, 7, 2445.
[3] Shanshan Chen, Yu Qi, Can Li, Kazunari Domen, Fuxiang Zhang*. Surface strategies for particulate photocatalysts towards artificial photosynthesis. Joule, 2018, 2, 2260.
[4] Shanshan Chen, Junie Jhon M. Vequizo, Zhenhua Pan, Takashi Hisatomi, Mamiko Nakabayashi, Lihua Lin, Zheng Wang, Kosaku Kato, Akira Yamakata, Naoya Shibata, Tsuyoshi Takata, Taro Yamada, Kazunari Domen*. Surface modifications of (ZnSe)0.5(CuGa2.5Se4.25)0.5 promoting photocatalytic Z-scheme overall water splitting. J. Am. Chem. Soc., 2021, 143, 10633.
[5] Shanshan Chen, Shuai Shen, Guiji Liu, Yu Qi, Fuxiang Zhang*, Can Li*. Interface engineering of CoOx/Ta3N5 photocatalyst for unprecedented water oxidation performance under visible light irradiation. Angew. Chem. Int. Ed.,2015, 54, 3047. (Highly cited paper)
[6] Shanshan Chen, Yu Qi, Takashi Hisatomi, Qian Ding, Tomohiro Asai, Zheng Li, Su Su Khine Ma, Fuxiang Zhang*, Kazunari Domen, Can Li*. Efficient visible-light-driven Z-scheme overall water splitting using a MgTa2O6−xNy/TaON heterostructure photocatalyst for H2 evolution. Angew. Chem. Int. Ed.,2015, 54, 8498.
[7] Shanshan Chen, Swarnava Nandy, Junie Jhon M. Vequizo, Takashi Hisatomi, Mamiko Nakabayashi, Zhenhua Pan, Qi Xiao, Zheng Wang, Lihua Lin, Song Sun, Kosaku Kato, Akira Yamakata, Naoya Shibata, Tsuyoshi Takata, Fuxiang Zhang, Kazunari Domen*. La5Ti2Cu0.9Ag0.1O7S5-based photocatalyst sheets for efficient Z-scheme overall water splitting. ACS Catal., 2023, 13, 3285.
[8] Shanshan Chen, Junie Jhon M. Vequizo, Takashi Hisatomi, Mamiko Nakabayashi, Lihua Lin, Zheng Wang, Akira Yamakata, Naoya Shibata, Tsuyoshi Takata, Taro Yamada, Kazunari Domen*. Efficient photocatalytic hydrogen evolution on single-crystalline metal selenide particles with suitable cocatalysts. Chem. Sci., 2020, 11, 6436. (HOT paper).
[9] Shanshan Chen, Guijun Ma, Qian Wang, Song Sun, Takashi Hisatomi, Tomohiro Higashi, Zheng Wang, Mamiko Nakabayashi, Naoya Shibata, Zhenhua Pan, Toshio Hayashi, Tsutomu Minegishi, Tsuyoshi Takata, Kazunari Domen*. Metal selenide photocatalysts for visible-light-driven Z-scheme pure water splitting. J. Mater. Chem. A, 2019, 7, 7415. (HOT paper)
[10] Shanshan Chen, Jingxiu Yang, Chunmei Ding, Rengui Li, Shaoqing Jin, Donge Wang, Hongxian Han, Fuxiang Zhang*, Can Li*. Nitrogen-doped layered oxide Sr5Ta4O15−xNx for water reduction and oxidation under visible light irradiation. J. Mater. Chem. A, 2013, 1, 5651.
[11] Shanshan Chen, Yu Qi, Qian Ding, Zheng Li, Junyan Cui, Fuxiang Zhang*, Can Li*. Magnesia interface nanolayer modification of Pt/Ta3N5 for promoted photocatalytic hydrogen production under visible light irradiation. J. Catal., 2016, 339, 77.
[12] Shanshan Chen, Yu Qi, Guiji Liu, Jingxiu Yang, Fuxiang Zhang*, Can Li*. A wide visible-light-responsive tunneled MgTa2O6–xNx photocatalyst for water oxidation and reduction. Chem. Commun., 2014, 50, 14415.
[13] Shanshan Chen, Takashi Hisatomi, Guijun Ma, Zheng Wang, Zhenhua Pan, Tsuyoshi Takata, Kazunari Domen*. Metal selenides for photocatalytic Z-scheme pure water splitting mediated by reduced graphene oxide. Chin. J. Catal., 2019, 40, 1668.
[14] Shanshan Chen, Fuxiang Zhang*. Recent progress on photocatalysts with wide visible light range absorption for heterogeneous water splitting. Chin. J. Catal., 2014, 35, 1431.
[15] Shanshan Chen, Yinhua Zhu, Wei Li, Weijia Liu, Licheng Li, Zhuhong Yang, Chang Liu, Wenjun Yao, Xiaohua Lu*, Xin Feng. Synthesis, features, and applications of mesoporous titania with TiO2(B). Chin. J. Catal., 2010, 31, 605.
[16] Zhongxu Yuan, Chunjiang Liu, Shanshan Chen*, Fuxiang Zhang*. Nanostructured (oxy)nitrides controllably synthesized by flux-assisted nitridation for promoted photocatalytic water splitting. J. Mater. Chem. A, 2024, 12, 5040.
[17] Huiqin An*, Yanjun Wang, Yu Ling, Zhiyao Ma, Xing Xiao, Tianxin Gao, Wanyu Hong, Lizhi Zhao, Hong Wang, Qingjun Zhu, Shanshan Chen*, Zhen Yin*. Photocatalytic seawater splitting on a plasmonic Au modified 2D heterostructure of ZnIn2S4/WO3 under visible light. J. Energy Chem., 2024, 93, 55.
[18] Ningning Wang, Shuo Wang, Can Li, Chenyang Li, Chunjiang Liu, Shanshan Chen*, Fuxiang Zhang*. ZrO2 modification of homogeneous nitrogen‐doped oxide MgTa2O6‒xNx for promoted photocatalytic water splitting. Chin. J. Catal., 2023, 54, 220.
[19] Can Li, Wenjun Fan, Shanshan Chen*, Fuxiang Zhang*. Effective charge carrier utilization of BiVO4 for solar overall water splitting. Chem. Eur. J., 2022, 28, e202201812.